223 research outputs found
Hopping magneto-transport via nonzero orbital momentum states and organic magnetoresistance
In hopping magnetoresistance of doped insulators, an applied magnetic field
shrinks the electron (hole) s-wave function of a donor or an acceptor and this
reduces the overlap between hopping sites resulting in the positive
magnetoresistance quadratic in a weak magnetic field, B. We extend the theory
of hopping magnetoresistance to states with nonzero orbital momenta. Different
from s-states, a weak magnetic field expands the electron (hole) wave functions
with positive magnetic quantum numbers, m > 0, and shrinks the states with
negative m in a wide region outside the point defect. This together with a
magnetic-field dependence of injection/ionization rates results in a negative
weak-field magnetoresistance, which is linear in B when the orbital degeneracy
is lifted. The theory provides a possible explanation of a large low-field
magnetoresistance in disordered pi-conjugated organic materials (OMAR).Comment: 4 pages, 3 figure
Ground state properties of ferromagnetic metal/conjugated polymer interfaces
We theoretically investigate the ground state properties of ferromagnetic
metal/conjugated polymer interfaces. The work is partially motivated by recent
experiments in which injection of spin polarized electrons from ferromagnetic
contacts into thin films of conjugated polymers was reported. We use a
one-dimensional nondegenerate Su-Schrieffer-Heeger (SSH) Hamiltonian to
describe the conjugated polymer and one-dimensional tight-binding models to
describe the ferromagnetic metal. We consider both a model for a conventional
ferromagnetic metal, in which there are no explicit structural degrees of
freedom, and a model for a half-metallic ferromagnetic colossal
magnetoresistance (CMR) oxide which has explicit structural degrees of freedom.
The Fermi energy of the magnetic metallic contact is adjusted to control the
degree of electron transfer into the polymer. We investigate electron charge
and spin transfer from the ferromagnetic metal to the organic polymer, and
structural relaxation near the interface. Bipolarons are the lowest energy
charge state in the bulk polymer for the nondegenerate SSH model Hamiltonian.
As a result electrons (or holes) transferred into the bulk of the polymer form
spinless bipolarons. However, there can be spin density in the polymer
localized near the interface.Comment: 7 figure
Erratum: “Seed layer technique for high quality epitaxial manganite films” [AIP Advances 6, 085109 (2016)]
No abstract available
Manganite/Alq3 interfaces investigated by impedance spectroscopy technique
With the general objective of studying interfaces between ferromagnetic materials and organic semiconductors, we report ac impedance investigations on La0.7Sr0.3MnO3 (LSMO)/tris(8-hydroxyquinoline)aluminium (Alq3)/Al and Indium Tin Oxide (ITO)/Alq3/Al heterostructures, in the frequency range between 20 Hz and 1 MHz. The comparison of the equivalent circuits deduced to fit the experimental ac responses allows isolating a specific RC contribution which can be attributed to the LSMO/Alq3 interface region. Using the information obtained from our ac measurements, we propose a model which fits the temperature dependence of the magnetoresistance in spin valves combining LSMO electrodes and Alq3 layers
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